Vertical distribution of plutonium isotopes from the floodplain and lacustrine sediments in Poyang Lake, China

Anthropogenic radionuclides deposited in sediments have been used for environmental radiation risk valuation as well as source identification. In this study, we investigated the vertical distribution of plutonium (Pu) isotopes and ²⁴⁰Pu/²³⁹Pu atom ratios in both floodplain and lacustrine sediments in Poyang Lake. The ^239+240Pu activity concentrations in floodplain sediment cores were found to range from 0.002 to 0.085 Bq kg⁻¹, with a maximum value at the subsurface layer. The activity in lacustrine sediment cores was from 0.062 to 0.351 Bq kg⁻¹ with a mean of 0.138 ± 0.053 Bq kg⁻¹. The inventory of 43.15 Bq m⁻² in lacustrine sediment core is comparable to the average value of global fallout expected at the same latitude. The average ²⁴⁰Pu/²³⁹Pu atomic ratios (0.183 ± 0.032) for sediment cores indicated that the global fallout is the major source of Pu in the studied region. The results are of great significance to the further understanding of sources, records, and environmental impacts of regional nuclear activities in the environment.