Time-Resolved X-Ray Diffraction: The Dynamics of the Chemical Bond

Research output: Chapter in Book/Report/Conference proceedingBook chapterResearchpeer-review

Abstract

We review the basic theoretical formulation for pulsed X-ray scattering on nonstationary molecular states. Relevant time scales are discussed for coherent as well as incpherent X-ray pulses. The general formalism is applied to a nonstationary diatomic molecule in order to highlight the relation between the signal and the time-dependent quamtum distribution of internuclear positions. Finally, a few experimental results are briefly discussed.
Original languageEnglish
Title of host publicationMolecular Electronic Structures of Transition Metal Complexes I
EditorsDavid Michael P. Mingos, Peter Day, Jens Peder Dahl
Number of pages215
PublisherSpringer
Publication date2012
Pages185-211
ISBN (Print)978-3-642-27370-4
Publication statusPublished - 2012
SeriesStructure and Bonding
Number142
ISSN0081-5993

Keywords

  • Inversion
  • Diatomic molecule
  • X-ray scattering
  • Nonstationary states
  • Pump probe

Cite this

Møller, K. B., & Henriksen, N. E. (2012). Time-Resolved X-Ray Diffraction: The Dynamics of the Chemical Bond. In D. M. P. Mingos, P. Day, & J. P. Dahl (Eds.), Molecular Electronic Structures of Transition Metal Complexes I (pp. 185-211). Springer. Structure and Bonding, No. 142
Møller, Klaus Braagaard ; Henriksen, Niels Engholm. / Time-Resolved X-Ray Diffraction: The Dynamics of the Chemical Bond. Molecular Electronic Structures of Transition Metal Complexes I. editor / David Michael P. Mingos ; Peter Day ; Jens Peder Dahl. Springer, 2012. pp. 185-211 (Structure and Bonding; No. 142).
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Møller, KB & Henriksen, NE 2012, Time-Resolved X-Ray Diffraction: The Dynamics of the Chemical Bond. in DMP Mingos, P Day & JP Dahl (eds), Molecular Electronic Structures of Transition Metal Complexes I. Springer, Structure and Bonding, no. 142, pp. 185-211.

Time-Resolved X-Ray Diffraction: The Dynamics of the Chemical Bond. / Møller, Klaus Braagaard; Henriksen, Niels Engholm.

Molecular Electronic Structures of Transition Metal Complexes I. ed. / David Michael P. Mingos; Peter Day; Jens Peder Dahl. Springer, 2012. p. 185-211 (Structure and Bonding; No. 142).

Research output: Chapter in Book/Report/Conference proceedingBook chapterResearchpeer-review

TY - CHAP

T1 - Time-Resolved X-Ray Diffraction: The Dynamics of the Chemical Bond

AU - Møller, Klaus Braagaard

AU - Henriksen, Niels Engholm

PY - 2012

Y1 - 2012

N2 - We review the basic theoretical formulation for pulsed X-ray scattering on nonstationary molecular states. Relevant time scales are discussed for coherent as well as incpherent X-ray pulses. The general formalism is applied to a nonstationary diatomic molecule in order to highlight the relation between the signal and the time-dependent quamtum distribution of internuclear positions. Finally, a few experimental results are briefly discussed.

AB - We review the basic theoretical formulation for pulsed X-ray scattering on nonstationary molecular states. Relevant time scales are discussed for coherent as well as incpherent X-ray pulses. The general formalism is applied to a nonstationary diatomic molecule in order to highlight the relation between the signal and the time-dependent quamtum distribution of internuclear positions. Finally, a few experimental results are briefly discussed.

KW - Inversion

KW - Diatomic molecule

KW - X-ray scattering

KW - Nonstationary states

KW - Pump probe

M3 - Book chapter

SN - 978-3-642-27370-4

SP - 185

EP - 211

BT - Molecular Electronic Structures of Transition Metal Complexes I

A2 - Mingos, David Michael P.

A2 - Day, Peter

A2 - Dahl, Jens Peder

PB - Springer

ER -

Møller KB, Henriksen NE. Time-Resolved X-Ray Diffraction: The Dynamics of the Chemical Bond. In Mingos DMP, Day P, Dahl JP, editors, Molecular Electronic Structures of Transition Metal Complexes I. Springer. 2012. p. 185-211. (Structure and Bonding; No. 142).