Theory of time-resolved inelastic x-ray diffraction

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Abstract

Starting from a general theory of time-resolved x-ray scattering, we derive a convenient expression for the diffraction signal based on a careful analysis of the relevant inelastic scattering processes. We demonstrate that the resulting inelastic limit applies to a wider variety of experimental conditions than similar, previously derived formulas, and it directly allows the application of selection rules when interpreting diffraction signals. Furthermore, we present a simple extension to systems simultaneously illuminated by x rays and a laser beam.
Original languageEnglish
JournalPhysical Review A
Volume81
Issue number2
Pages (from-to)023422
ISSN2469-9926
DOIs
Publication statusPublished - 2010

Bibliographical note

Copyright 2010 American Physical Society

Cite this

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title = "Theory of time-resolved inelastic x-ray diffraction",
abstract = "Starting from a general theory of time-resolved x-ray scattering, we derive a convenient expression for the diffraction signal based on a careful analysis of the relevant inelastic scattering processes. We demonstrate that the resulting inelastic limit applies to a wider variety of experimental conditions than similar, previously derived formulas, and it directly allows the application of selection rules when interpreting diffraction signals. Furthermore, we present a simple extension to systems simultaneously illuminated by x rays and a laser beam.",
author = "Ulf Lorenz and M{\o}ller, {Klaus Braagaard} and Henriksen, {Niels Engholm}",
note = "Copyright 2010 American Physical Society",
year = "2010",
doi = "10.1103/PhysRevA.81.023422",
language = "English",
volume = "81",
pages = "023422",
journal = "Physical Review A (Atomic, Molecular and Optical Physics)",
issn = "2469-9926",
publisher = "American Physical Society",
number = "2",

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Theory of time-resolved inelastic x-ray diffraction. / Lorenz, Ulf; Møller, Klaus Braagaard; Henriksen, Niels Engholm.

In: Physical Review A, Vol. 81, No. 2, 2010, p. 023422.

Research output: Contribution to journalJournal articleResearchpeer-review

TY - JOUR

T1 - Theory of time-resolved inelastic x-ray diffraction

AU - Lorenz, Ulf

AU - Møller, Klaus Braagaard

AU - Henriksen, Niels Engholm

N1 - Copyright 2010 American Physical Society

PY - 2010

Y1 - 2010

N2 - Starting from a general theory of time-resolved x-ray scattering, we derive a convenient expression for the diffraction signal based on a careful analysis of the relevant inelastic scattering processes. We demonstrate that the resulting inelastic limit applies to a wider variety of experimental conditions than similar, previously derived formulas, and it directly allows the application of selection rules when interpreting diffraction signals. Furthermore, we present a simple extension to systems simultaneously illuminated by x rays and a laser beam.

AB - Starting from a general theory of time-resolved x-ray scattering, we derive a convenient expression for the diffraction signal based on a careful analysis of the relevant inelastic scattering processes. We demonstrate that the resulting inelastic limit applies to a wider variety of experimental conditions than similar, previously derived formulas, and it directly allows the application of selection rules when interpreting diffraction signals. Furthermore, we present a simple extension to systems simultaneously illuminated by x rays and a laser beam.

U2 - 10.1103/PhysRevA.81.023422

DO - 10.1103/PhysRevA.81.023422

M3 - Journal article

VL - 81

SP - 023422

JO - Physical Review A (Atomic, Molecular and Optical Physics)

JF - Physical Review A (Atomic, Molecular and Optical Physics)

SN - 2469-9926

IS - 2

ER -