The influence of static pre-stretching on the mechanical ageing of filled silicone rubbers for dielectric elastomer applications

Shamsul Bin Zakaria, Liyun Yu, Guggi Kofod, Anne Ladegaard Skov

Research output: Contribution to journalJournal articleResearchpeer-review

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Abstract

Dielectric elastomer (DE) pre-stretching is a key aspect of attaining better actuation performance, as ithelps prevent electromechanical instability (EMI) and usually lowers the Young’s modulus, thus leading toeasier deformation. The pre-stretched DE is not only susceptible to a high risk of tearing and the formationof mechanical defects, but films with sustained and substantial strain may also experience mechanicaldegradation. In this study a long-term mechanical reliability study of DE is performed. Young’s mod-uli, dielectric breakdown strengths and dielectric permittivities of commercial silica-reinforced siliconeelastomers, with and without an additional 35% (35 phr) of titanium dioxide (TiO2), were investigatedafter being subjected to pre-stretching for various timespans at pre-stretches to strains of 60 and 120%,respectively. The study shows that mechanical stability when pre-stretching is difficult to achieve withhighly filled elastomers. However, despite the negative outlook for metal oxide-filled silicone elastomers,the study paves the way for reliable dielectric elastomers by indicating that simply post-curing siliconeelastomers before use may increase reliability.
Original languageEnglish
JournalMaterials Today Communications
Volume4
Pages (from-to)204-213
ISSN2352-4928
DOIs
Publication statusPublished - 2015

Keywords

  • Pre-stretching
  • Mechanical ageing
  • Silicone composite
  • PDMS
  • Dielectric elastomera

Cite this

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title = "The influence of static pre-stretching on the mechanical ageing of filled silicone rubbers for dielectric elastomer applications",
abstract = "Dielectric elastomer (DE) pre-stretching is a key aspect of attaining better actuation performance, as ithelps prevent electromechanical instability (EMI) and usually lowers the Young’s modulus, thus leading toeasier deformation. The pre-stretched DE is not only susceptible to a high risk of tearing and the formationof mechanical defects, but films with sustained and substantial strain may also experience mechanicaldegradation. In this study a long-term mechanical reliability study of DE is performed. Young’s mod-uli, dielectric breakdown strengths and dielectric permittivities of commercial silica-reinforced siliconeelastomers, with and without an additional 35{\%} (35 phr) of titanium dioxide (TiO2), were investigatedafter being subjected to pre-stretching for various timespans at pre-stretches to strains of 60 and 120{\%},respectively. The study shows that mechanical stability when pre-stretching is difficult to achieve withhighly filled elastomers. However, despite the negative outlook for metal oxide-filled silicone elastomers,the study paves the way for reliable dielectric elastomers by indicating that simply post-curing siliconeelastomers before use may increase reliability.",
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The influence of static pre-stretching on the mechanical ageing of filled silicone rubbers for dielectric elastomer applications. / Zakaria, Shamsul Bin; Yu, Liyun; Kofod, Guggi; Skov, Anne Ladegaard.

In: Materials Today Communications, Vol. 4, 2015, p. 204-213.

Research output: Contribution to journalJournal articleResearchpeer-review

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T1 - The influence of static pre-stretching on the mechanical ageing of filled silicone rubbers for dielectric elastomer applications

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AU - Kofod, Guggi

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PY - 2015

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