Terahertz-induced Kerr effect in amorphous chalcogenide glasses

Maksim Zalkovskij, Andrew Strikwerda, Krzysztof Iwaszczuk, A. Popescu, A. Savastru, Radu Malureanu, Andrei Lavrinenko, Peter Uhd Jepsen

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    Abstract

    We have investigated the terahertz-induced third-order (Kerr) nonlinear optical properties of the amorphous chalcogenide glasses As2S3 and As2Se3. Chalcogenide glasses are known for their high optical Kerr nonlinearities which can be several hundred times greater than those of fused silica. We use high-intensity, single-cycle terahertz pulses with a maximum electrical field strength exceeding 400 kV/cm and frequency content from 0.2 to 3.0 THz. By optical Kerr-gate sampling, we measured the terahertz-induced nonlinear refractive indices at 800nm to be n2 = 1.746 x 10-14 cm2/W for As2S3 and n2 = 3.440 x 10-14 cm2/W for As2Se3.
    Original languageEnglish
    Article number221102
    JournalApplied Physics Letters
    Volume103
    Issue number22
    Number of pages4
    ISSN0003-6951
    DOIs
    Publication statusPublished - 2013

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