Separation of Flue Gas Components by SILP (Supported Ionic Liquid-Phase) Absorbers

P. Thomassen, Andreas Jonas Kunov-Kruse, Susanne L. Mossin, Helene Kolding, Søren Kegnæs, Anders Riisager, Rasmus Fehrmann

Research output: Contribution to journalConference articleResearchpeer-review

Abstract

Reversible absorption of the flue gas components CO2, NO, NO2 and SO2 has been tested for different ionic liquids (ILs) at different temperatures and flue gas compositions where porous, high surface area carriers have been applied as supports for the ionic liquids to obtain Supported Ionic Liquid-Phase (SILP) absorber materials. The use of solid SILP absorbers with selected ILs were found to significantly improve the absorption capacity and sorption dynamics at low flue gas concentration, thus making the applicability of ILs viable in technical, continuous flow processes for flue gas cleaning. The results show that CO2, NO and SO2 can be reversible and selective absorbed using different ILs and that Supported Ionic Liquid-Phase (SILP) absorbers are promising materials for industrial flue gas cleaning. Absorption/desorption dynamics can be tuned by temperature, pressure and gas concentration.

© 2012 ECS - The Electrochemical Society
Original languageEnglish
JournalE C S Transactions
Volume50
Issue number11
Pages (from-to)433-442
ISSN1938-5862
DOIs
Publication statusPublished - 2013
EventPacific Rim Meeting on Electrochemical and Solid-State Science: 222nd Meeting of ECS — The Electrochemical Society and 2012 Fall Meeting of The Electrochemical Society of Japan - Hawaii Convention Center and the Hilton Hawaiian Village, Honolulu, United States
Duration: 7 Oct 201212 Oct 2012
http://www.electrochem.org/meetings/biannual/222/222.htm

Conference

ConferencePacific Rim Meeting on Electrochemical and Solid-State Science
LocationHawaii Convention Center and the Hilton Hawaiian Village
CountryUnited States
CityHonolulu
Period07/10/201212/10/2012
Internet address

Cite this

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title = "Separation of Flue Gas Components by SILP (Supported Ionic Liquid-Phase) Absorbers",
abstract = "Reversible absorption of the flue gas components CO2, NO, NO2 and SO2 has been tested for different ionic liquids (ILs) at different temperatures and flue gas compositions where porous, high surface area carriers have been applied as supports for the ionic liquids to obtain Supported Ionic Liquid-Phase (SILP) absorber materials. The use of solid SILP absorbers with selected ILs were found to significantly improve the absorption capacity and sorption dynamics at low flue gas concentration, thus making the applicability of ILs viable in technical, continuous flow processes for flue gas cleaning. The results show that CO2, NO and SO2 can be reversible and selective absorbed using different ILs and that Supported Ionic Liquid-Phase (SILP) absorbers are promising materials for industrial flue gas cleaning. Absorption/desorption dynamics can be tuned by temperature, pressure and gas concentration.{\circledC} 2012 ECS - The Electrochemical Society",
author = "P. Thomassen and Kunov-Kruse, {Andreas Jonas} and Mossin, {Susanne L.} and Helene Kolding and S{\o}ren Kegn{\ae}s and Anders Riisager and Rasmus Fehrmann",
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doi = "10.1149/05011.0433ecst",
language = "English",
volume = "50",
pages = "433--442",
journal = "E C S Transactions",
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Separation of Flue Gas Components by SILP (Supported Ionic Liquid-Phase) Absorbers. / Thomassen, P.; Kunov-Kruse, Andreas Jonas; Mossin, Susanne L.; Kolding, Helene; Kegnæs, Søren; Riisager, Anders; Fehrmann, Rasmus.

In: E C S Transactions, Vol. 50, No. 11, 2013, p. 433-442.

Research output: Contribution to journalConference articleResearchpeer-review

TY - GEN

T1 - Separation of Flue Gas Components by SILP (Supported Ionic Liquid-Phase) Absorbers

AU - Thomassen, P.

AU - Kunov-Kruse, Andreas Jonas

AU - Mossin, Susanne L.

AU - Kolding, Helene

AU - Kegnæs, Søren

AU - Riisager, Anders

AU - Fehrmann, Rasmus

PY - 2013

Y1 - 2013

N2 - Reversible absorption of the flue gas components CO2, NO, NO2 and SO2 has been tested for different ionic liquids (ILs) at different temperatures and flue gas compositions where porous, high surface area carriers have been applied as supports for the ionic liquids to obtain Supported Ionic Liquid-Phase (SILP) absorber materials. The use of solid SILP absorbers with selected ILs were found to significantly improve the absorption capacity and sorption dynamics at low flue gas concentration, thus making the applicability of ILs viable in technical, continuous flow processes for flue gas cleaning. The results show that CO2, NO and SO2 can be reversible and selective absorbed using different ILs and that Supported Ionic Liquid-Phase (SILP) absorbers are promising materials for industrial flue gas cleaning. Absorption/desorption dynamics can be tuned by temperature, pressure and gas concentration.© 2012 ECS - The Electrochemical Society

AB - Reversible absorption of the flue gas components CO2, NO, NO2 and SO2 has been tested for different ionic liquids (ILs) at different temperatures and flue gas compositions where porous, high surface area carriers have been applied as supports for the ionic liquids to obtain Supported Ionic Liquid-Phase (SILP) absorber materials. The use of solid SILP absorbers with selected ILs were found to significantly improve the absorption capacity and sorption dynamics at low flue gas concentration, thus making the applicability of ILs viable in technical, continuous flow processes for flue gas cleaning. The results show that CO2, NO and SO2 can be reversible and selective absorbed using different ILs and that Supported Ionic Liquid-Phase (SILP) absorbers are promising materials for industrial flue gas cleaning. Absorption/desorption dynamics can be tuned by temperature, pressure and gas concentration.© 2012 ECS - The Electrochemical Society

U2 - 10.1149/05011.0433ecst

DO - 10.1149/05011.0433ecst

M3 - Conference article

VL - 50

SP - 433

EP - 442

JO - E C S Transactions

JF - E C S Transactions

SN - 1938-5862

IS - 11

ER -