Abstract
| Original language | English |
|---|---|
| Journal | Journal of Physical Chemistry Part B: Condensed Matter, Materials, Surfaces, Interfaces & Biophysical, The |
| Volume | 112 |
| Issue number | 2 |
| Pages (from-to) | 558-567 |
| ISSN | 1520-6106 |
| DOIs | |
| Publication status | Published - 2008 |
Cite this
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On the theory of time-resolved x-ray diffraction. / Henriksen, Niels Engholm; Møller, Klaus Braagaard.
In: Journal of Physical Chemistry Part B: Condensed Matter, Materials, Surfaces, Interfaces & Biophysical, The, Vol. 112, No. 2, 2008, p. 558-567.Research output: Contribution to journal › Journal article › Research › peer-review
TY - JOUR
T1 - On the theory of time-resolved x-ray diffraction
AU - Henriksen, Niels Engholm
AU - Møller, Klaus Braagaard
PY - 2008
Y1 - 2008
N2 - We derive the basic theoretical formulation for X-ray diffraction with pulsed fields, using a fully quantized description of light and matter. Relevant time scales are discussed for coherent as well as incoherent X-ray pulses, and we provide expressions to be used for calculation of the experimental diffraction signal for both types of X-ray sources. We present a simple analysis of time-resolved X-ray scattering for direct bond breaking in diatomic molecules. This essentially analytical approach highlights the relation between the signal and the time-dependent quantum distribution of internuclear positions, including thermal effects.
AB - We derive the basic theoretical formulation for X-ray diffraction with pulsed fields, using a fully quantized description of light and matter. Relevant time scales are discussed for coherent as well as incoherent X-ray pulses, and we provide expressions to be used for calculation of the experimental diffraction signal for both types of X-ray sources. We present a simple analysis of time-resolved X-ray scattering for direct bond breaking in diatomic molecules. This essentially analytical approach highlights the relation between the signal and the time-dependent quantum distribution of internuclear positions, including thermal effects.
U2 - 10.1021/jp075497e
DO - 10.1021/jp075497e
M3 - Journal article
VL - 112
SP - 558
EP - 567
JO - Journal of Physical Chemistry Part B: Condensed Matter, Materials, Surfaces, Interfaces & Biophysical
JF - Journal of Physical Chemistry Part B: Condensed Matter, Materials, Surfaces, Interfaces & Biophysical
SN - 1520-6106
IS - 2
ER -