On the application of ICP-MS techniques for measuring uranium and plutonium: a Nordic inter-laboratory comparison exercise

Jixin Qiao; Petra Lagerkvist; Ilia  Rodushkin; Susanna Salminen-Paatero; Per Roos; Syverin  Lierhagen; Karl Andreas  Jensen; Emma  Engstrom; Yann  Lahaye; Lindis  Skipperud

doi:10.1007/s10967-018-5697-4

On the application of ICP-MS techniques for measuring uranium and plutonium: a Nordic inter-laboratory comparison exercise

Jixin Qiao^*, Petra Lagerkvist, Ilia Rodushkin, Susanna Salminen-Paatero, Per Roos, Syverin Lierhagen, Karl Andreas Jensen, Emma Engstrom, Yann Lahaye, Lindis Skipperud

^*Corresponding author for this work

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Abstract

Inductively coupled plasma mass spectrometry (ICP-MS) techniques are widely used for determination of long-lived radionuclides and their isotopic ratios in the nuclear fields. Uranium (U) and Pu (Pu) isotopes have been determined by many researchers with ICP-MS due to its relatively high sensitivity and short measurement time. In this work, an inter-laboratory comparison exercise among the Nordic countries was performed, focusing on the measurement of U and Pu isotopes in certified reference materials by ICP-MS. The performance and characters of different ICP-MS instruments are evaluated and discussed in this paper.

Original language	English
Journal	Journal of Radioanalytical and Nuclear Chemistry
Volume	315
Issue number	3
Pages (from-to)	565-580
ISSN	0236-5731
DOIs	https://doi.org/10.1007/s10967-018-5697-4
Publication status	Published - 2018

Keywords

ICP-MS
Pu
U
NBL CRM-103A
IAEA-384

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Jixin ICP MS intercomparison revision submittedAccepted author manuscript, 840 KB

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Qiao, J., Lagerkvist, P., Rodushkin, I., Salminen-Paatero, S., Roos, P., Lierhagen, S., Jensen, K. A., Engstrom, E., Lahaye, Y., & Skipperud, L. (2018). On the application of ICP-MS techniques for measuring uranium and plutonium: a Nordic inter-laboratory comparison exercise. Journal of Radioanalytical and Nuclear Chemistry, 315(3), 565-580. https://doi.org/10.1007/s10967-018-5697-4

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abstract = "Inductively coupled plasma mass spectrometry (ICP-MS) techniques are widely used for determination of long-lived radionuclides and their isotopic ratios in the nuclear fields. Uranium (U) and Pu (Pu) isotopes have been determined by many researchers with ICP-MS due to its relatively high sensitivity and short measurement time. In this work, an inter-laboratory comparison exercise among the Nordic countries was performed, focusing on the measurement of U and Pu isotopes in certified reference materials by ICP-MS. The performance and characters of different ICP-MS instruments are evaluated and discussed in this paper. ",

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author = "Jixin Qiao and Petra Lagerkvist and Ilia Rodushkin and Susanna Salminen-Paatero and Per Roos and Syverin Lierhagen and Jensen, {Karl Andreas} and Emma Engstrom and Yann Lahaye and Lindis Skipperud",

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Qiao, J, Lagerkvist, P, Rodushkin, I, Salminen-Paatero, S, Roos, P, Lierhagen, S, Jensen, KA, Engstrom, E, Lahaye, Y & Skipperud, L 2018, 'On the application of ICP-MS techniques for measuring uranium and plutonium: a Nordic inter-laboratory comparison exercise', Journal of Radioanalytical and Nuclear Chemistry, vol. 315, no. 3, pp. 565-580. https://doi.org/10.1007/s10967-018-5697-4

TY - JOUR

T1 - On the application of ICP-MS techniques for measuring uranium and plutonium: a Nordic inter-laboratory comparison exercise

AU - Qiao, Jixin

AU - Lagerkvist, Petra

AU - Rodushkin, Ilia

AU - Salminen-Paatero, Susanna

AU - Roos, Per

AU - Lierhagen, Syverin

AU - Jensen, Karl Andreas

AU - Engstrom, Emma

AU - Lahaye, Yann

AU - Skipperud, Lindis

PY - 2018

Y1 - 2018

N2 - Inductively coupled plasma mass spectrometry (ICP-MS) techniques are widely used for determination of long-lived radionuclides and their isotopic ratios in the nuclear fields. Uranium (U) and Pu (Pu) isotopes have been determined by many researchers with ICP-MS due to its relatively high sensitivity and short measurement time. In this work, an inter-laboratory comparison exercise among the Nordic countries was performed, focusing on the measurement of U and Pu isotopes in certified reference materials by ICP-MS. The performance and characters of different ICP-MS instruments are evaluated and discussed in this paper.

AB - Inductively coupled plasma mass spectrometry (ICP-MS) techniques are widely used for determination of long-lived radionuclides and their isotopic ratios in the nuclear fields. Uranium (U) and Pu (Pu) isotopes have been determined by many researchers with ICP-MS due to its relatively high sensitivity and short measurement time. In this work, an inter-laboratory comparison exercise among the Nordic countries was performed, focusing on the measurement of U and Pu isotopes in certified reference materials by ICP-MS. The performance and characters of different ICP-MS instruments are evaluated and discussed in this paper.

KW - ICP-MS

KW - Pu

KW - U

KW - NBL CRM-103A

KW - IAEA-384

U2 - 10.1007/s10967-018-5697-4

DO - 10.1007/s10967-018-5697-4

M3 - Journal article

SN - 0236-5731

VL - 315

SP - 565

EP - 580

JO - Journal of Radioanalytical and Nuclear Chemistry

JF - Journal of Radioanalytical and Nuclear Chemistry

IS - 3

ER -

On the application of ICP-MS techniques for measuring uranium and plutonium: a Nordic inter-laboratory comparison exercise

Abstract

Keywords

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