Nonlinear Dynamics of Ultrashort Long-Range Surface Plasmon Polariton Pulses in Gold Strip Waveguides

Oleg Lysenko, Morten Bache, Nicolas Olivier, Anatoly V. Zayats, Andrei Lavrinenko

    Research output: Contribution to journalJournal articleResearchpeer-review

    241 Downloads (Pure)

    Abstract

    We study experimentally and theoretically nonlinear propagation of ultrashort long-range surface plasmon polaritons in gold strip waveguides. The nonlinear absorption of the plasmonic modes in the waveguides is measured with femtosecond pulses revealing a strong dependence of the third-order nonlinear susceptibility of the gold core on the pulse duration and layer thickness. A comprehensive model for the pulse duration dependence of the third-order nonlinear susceptibility is developed on the basis of the nonlinear Schrödinger equation for plasmonic mode propagation in the waveguides. The model accounts for the intrinsic delayed (noninstantaneous) nonlinearity of free electrons of gold as well as the thickness of the gold film and is experimentally verified. The obtained results are important for the development of active plasmonic and nanophotonic components.
    Original languageEnglish
    JournalACS Photonics
    Volume3
    Issue number12
    Pages (from-to)2324-2329
    ISSN2330-4022
    DOIs
    Publication statusPublished - 2016

    Keywords

    • plasmonics
    • nonlinear optics
    • ultrafast nonlinearity

    Fingerprint

    Dive into the research topics of 'Nonlinear Dynamics of Ultrashort Long-Range Surface Plasmon Polariton Pulses in Gold Strip Waveguides'. Together they form a unique fingerprint.

    Cite this