Joining of ceramic Ba0.5Sr0.5Co0.8Fe0.2O3 membranes for oxygen production to high temperature alloys

Wolff-Ragnar Kiebach; Kurt Engelbrecht; Kawai Kwok; Sebastian Molin; Martin Søgaard; Patrick Niehoff; Falk Schulze-Küppers; Ralf Kriegel; Jens Kluge; Peter Vang Hendriksen

doi:10.1016/j.memsci.2016.01.050

Joining of ceramic Ba_0.5Sr_0.5Co_0.8Fe_0.2O₃ membranes for oxygen production to high temperature alloys

Wolff-Ragnar Kiebach
, Kurt Engelbrecht
, Kawai Kwok
, Sebastian Molin
, Martin Søgaard
, Patrick Niehoff
, Falk Schulze-Küppers
, Ralf Kriegel
, Jens Kluge
, Peter Vang Hendriksen

Department of Energy Conversion and Storage

Research output: Contribution to journal › Journal article › Research › peer-review

Abstract

The possibility of joining dense ceramic BCSF tubular membranes to metal alloys using a silver braze was investigated. Four different alloys (Crofer 22 APU (R), Kanthal APM (R), Haynes 214 (R) and EN 1.4841) were considered and the influence of their oxide scale stability/reactivity and their thermal expansion coefficient on the stability of the final joint was evaluated. Leak tight assemblies were obtained only for steels with a thermal expansion coefficient of > 16 [10(-6) K-1] and protective coating. Proof-of-concept oxygen flux measurements up to 830 degrees C were performed on these assemblies, demonstrating the functionality of the developed hot sealing. In addition a simulation of the stresses occurring in the joint assembly during use was performed for different materials and geometries. The obtained results fit well with the experimental findings. (C) 2016 Elsevier B.V. All rights reserved.

Original language	English
Journal	Journal of Membrane Science
Volume	506
Pages (from-to)	11-21
Number of pages	11
ISSN	0376-7388
DOIs	https://doi.org/10.1016/j.memsci.2016.01.050
Publication status	Published - 2016

Keywords

Brazing
BSCF
Carbon capture and sequestration
Joining ceramic to metal
Oxygen transport membrane

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10.1016/j.memsci.2016.01.050

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@article{62408899c43449879f12df28814e4034,

title = "Joining of ceramic Ba0.5Sr0.5Co0.8Fe0.2O3 membranes for oxygen production to high temperature alloys",

abstract = "The possibility of joining dense ceramic BCSF tubular membranes to metal alloys using a silver braze was investigated. Four different alloys (Crofer 22 APU (R), Kanthal APM (R), Haynes 214 (R) and EN 1.4841) were considered and the influence of their oxide scale stability/reactivity and their thermal expansion coefficient on the stability of the final joint was evaluated. Leak tight assemblies were obtained only for steels with a thermal expansion coefficient of > 16 [10(-6) K-1] and protective coating. Proof-of-concept oxygen flux measurements up to 830 degrees C were performed on these assemblies, demonstrating the functionality of the developed hot sealing. In addition a simulation of the stresses occurring in the joint assembly during use was performed for different materials and geometries. The obtained results fit well with the experimental findings. (C) 2016 Elsevier B.V. All rights reserved.",

keywords = "Brazing, BSCF, Carbon capture and sequestration, Joining ceramic to metal, Oxygen transport membrane",

author = "Wolff-Ragnar Kiebach and Kurt Engelbrecht and Kawai Kwok and Sebastian Molin and Martin S{\o}gaard and Patrick Niehoff and Falk Schulze-K{\"u}ppers and Ralf Kriegel and Jens Kluge and Hendriksen, \{Peter Vang\}",

year = "2016",

doi = "10.1016/j.memsci.2016.01.050",

language = "English",

volume = "506",

pages = "11--21",

journal = "Journal of Membrane Science",

issn = "0376-7388",

publisher = "Elsevier",

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TY - JOUR

T1 - Joining of ceramic Ba0.5Sr0.5Co0.8Fe0.2O3 membranes for oxygen production to high temperature alloys

AU - Kiebach, Wolff-Ragnar

AU - Engelbrecht, Kurt

AU - Kwok, Kawai

AU - Molin, Sebastian

AU - Søgaard, Martin

AU - Niehoff, Patrick

AU - Schulze-Küppers, Falk

AU - Kriegel, Ralf

AU - Kluge, Jens

AU - Hendriksen, Peter Vang

PY - 2016

Y1 - 2016

N2 - The possibility of joining dense ceramic BCSF tubular membranes to metal alloys using a silver braze was investigated. Four different alloys (Crofer 22 APU (R), Kanthal APM (R), Haynes 214 (R) and EN 1.4841) were considered and the influence of their oxide scale stability/reactivity and their thermal expansion coefficient on the stability of the final joint was evaluated. Leak tight assemblies were obtained only for steels with a thermal expansion coefficient of > 16 [10(-6) K-1] and protective coating. Proof-of-concept oxygen flux measurements up to 830 degrees C were performed on these assemblies, demonstrating the functionality of the developed hot sealing. In addition a simulation of the stresses occurring in the joint assembly during use was performed for different materials and geometries. The obtained results fit well with the experimental findings. (C) 2016 Elsevier B.V. All rights reserved.

AB - The possibility of joining dense ceramic BCSF tubular membranes to metal alloys using a silver braze was investigated. Four different alloys (Crofer 22 APU (R), Kanthal APM (R), Haynes 214 (R) and EN 1.4841) were considered and the influence of their oxide scale stability/reactivity and their thermal expansion coefficient on the stability of the final joint was evaluated. Leak tight assemblies were obtained only for steels with a thermal expansion coefficient of > 16 [10(-6) K-1] and protective coating. Proof-of-concept oxygen flux measurements up to 830 degrees C were performed on these assemblies, demonstrating the functionality of the developed hot sealing. In addition a simulation of the stresses occurring in the joint assembly during use was performed for different materials and geometries. The obtained results fit well with the experimental findings. (C) 2016 Elsevier B.V. All rights reserved.

KW - Brazing

KW - BSCF

KW - Carbon capture and sequestration

KW - Joining ceramic to metal

KW - Oxygen transport membrane

U2 - 10.1016/j.memsci.2016.01.050

DO - 10.1016/j.memsci.2016.01.050

M3 - Journal article

SN - 0376-7388

VL - 506

SP - 11

EP - 21

JO - Journal of Membrane Science

JF - Journal of Membrane Science

ER -