Abstract
We measure 3H in an ice core from Camp Century. The temporal distribution of 3H
concentration in the ice core corresponds generally well with the
historical record of explosive yields of atmospheric nuclear weapons
tests. Maximum 3H values observed in 1962–1963 are comparable
to those in ice core or precipitation in many other locations in the
Northern Hemisphere. There is no indication that significant 3H
contamination was locally released into the air during the operation of
the Camp Century reactor. It is, however, somewhat surprising that
several prominent 3H peaks are still observed after 1980. We suggest that these are associated with airborne 3H
releases from the civil nuclear industry. A wavelet analysis during
1970–2017 indicates the primary frequency of variability in the 3H record is annual 3H peaks. These annual peaks can be combined with the 3H
spikes from global fallout of known nuclear weapons tests to benchmark
and evaluate theoretical ice core dating scales back to the 1950s. A
positive correlation is observed between annual 3H average concentration and variability of Arctic Oscillation (AO). This highlights the value of 3H as a potential tracer for air masses and airborne pollutants in the Arctic.
| Original language | English |
|---|---|
| Journal | Environmental Science and Technology |
| Volume | 55 |
| Pages (from-to) | 13638−13645 |
| ISSN | 0013-936X |
| DOIs | |
| Publication status | Published - 2021 |
Keywords
- Camp Century
- Ice core
- Source
- Tracer application
- Tritium
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