Experimental validation of a rate-based model for CO2 capture using an AMP solution

Jostein Gabrielsen; H. F. Svendsen; Michael Locht Michelsen; Erling Halfdan Stenby; Georgios Kontogeorgis

doi:10.1016/j.ces.2007.01.034

Experimental validation of a rate-based model for CO2 capture using an AMP solution

Jostein Gabrielsen
, H. F. Svendsen
, Michael Locht Michelsen
, Erling Halfdan Stenby
, Georgios Kontogeorgis

Research output: Contribution to journal › Journal article › Research › peer-review

Abstract

Detailed experimental data, including temperature profiles over the absorber, for a carbon dioxide (CO"2) absorber with structured packing in an integrated laboratory pilot plant using an aqueous 2-amino-2-methyl-1-propanol (AMP) solution are presented. The experimental gas-liquid material balance was within an average of 3.5% for the experimental conditions presented. A predictive rate-based steady-state model for CO"2 absorption into an AMP solution, using an implicit expression for the enhancement factor, has been validated against the presented pilot plant data. Furthermore, a parameter sensitivity analysis for the proposed model has been carried out.

Original language	English
Journal	Chemical Engineering Science
Volume	62
Issue number	9
Pages (from-to)	2397-2413
ISSN	0009-2509
DOIs	https://doi.org/10.1016/j.ces.2007.01.034
Publication status	Published - 2007

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title = "Experimental validation of a rate-based model for CO2 capture using an AMP solution",

abstract = "Detailed experimental data, including temperature profiles over the absorber, for a carbon dioxide (CO{"}2) absorber with structured packing in an integrated laboratory pilot plant using an aqueous 2-amino-2-methyl-1-propanol (AMP) solution are presented. The experimental gas-liquid material balance was within an average of 3.5\% for the experimental conditions presented. A predictive rate-based steady-state model for CO{"}2 absorption into an AMP solution, using an implicit expression for the enhancement factor, has been validated against the presented pilot plant data. Furthermore, a parameter sensitivity analysis for the proposed model has been carried out.",

author = "Jostein Gabrielsen and Svendsen, \{H. F.\} and Michelsen, \{Michael Locht\} and Stenby, \{Erling Halfdan\} and Georgios Kontogeorgis",

year = "2007",

doi = "10.1016/j.ces.2007.01.034",

language = "English",

volume = "62",

pages = "2397--2413",

journal = "Chemical Engineering Science",

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T1 - Experimental validation of a rate-based model for CO2 capture using an AMP solution

AU - Gabrielsen, Jostein

AU - Svendsen, H. F.

AU - Michelsen, Michael Locht

AU - Stenby, Erling Halfdan

AU - Kontogeorgis, Georgios

PY - 2007

Y1 - 2007

N2 - Detailed experimental data, including temperature profiles over the absorber, for a carbon dioxide (CO"2) absorber with structured packing in an integrated laboratory pilot plant using an aqueous 2-amino-2-methyl-1-propanol (AMP) solution are presented. The experimental gas-liquid material balance was within an average of 3.5% for the experimental conditions presented. A predictive rate-based steady-state model for CO"2 absorption into an AMP solution, using an implicit expression for the enhancement factor, has been validated against the presented pilot plant data. Furthermore, a parameter sensitivity analysis for the proposed model has been carried out.

AB - Detailed experimental data, including temperature profiles over the absorber, for a carbon dioxide (CO"2) absorber with structured packing in an integrated laboratory pilot plant using an aqueous 2-amino-2-methyl-1-propanol (AMP) solution are presented. The experimental gas-liquid material balance was within an average of 3.5% for the experimental conditions presented. A predictive rate-based steady-state model for CO"2 absorption into an AMP solution, using an implicit expression for the enhancement factor, has been validated against the presented pilot plant data. Furthermore, a parameter sensitivity analysis for the proposed model has been carried out.

U2 - 10.1016/j.ces.2007.01.034

DO - 10.1016/j.ces.2007.01.034

M3 - Journal article

SN - 0009-2509

VL - 62

SP - 2397

EP - 2413

JO - Chemical Engineering Science

JF - Chemical Engineering Science

IS - 9

ER -

Experimental validation of a rate-based model for CO2 capture using an AMP solution

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