Electron transport in nanoporous graphene: Probing the Talbot effect

Gaetano Calogero, Nick Rübner Papior, Bernhard Kretz, Aran Garcia-Lekue, Thomas Frederiksen, Mads Brandbyge*

*Corresponding author for this work

Research output: Contribution to journalJournal articleResearchpeer-review

Abstract

Electrons in graphene can show diffraction and interference phenomena fully analogous to light thanks to their Dirac-like energy dispersion. However it is not clear how this optical analogy persists in nanostructured graphene, e.g. with pores. Nanoporous graphene (NPG) consisting of linked graphene nanoribbons has recently been fabricated using molecular precursors and bottom-up assembly [Moreno et al, Science 360, 199 (2018)]. We predict that electrons propagating in NPG exhibit the interference Talbot effect, analogous to photons in coupled waveguides. Our results are obtained by parameter-free atomistic calculations of real-sized NPG samples, based on seamlessly integrated density functional theory and tight-binding regions. We link the origins of this interference phenomenon to the band structure of the NPG. Most importantly, we demonstrate how the Talbot effect may be detected experimentally using dual-probe scanning tunneling microscopy. Talbot interference of electron waves in NPG or other related materials may open up new opportunities for future quantum electronics, computing or sensing.
Original languageEnglish
JournalNano letters
Volume19
Issue number1
Pages (from-to)576-581
Number of pages6
ISSN1530-6984
DOIs
Publication statusPublished - 2019

Keywords

  • Nanoporous graphene
  • Talbot interference
  • Electron transport
  • Scanning probe microscopy
  • Multiscale modeling

Cite this

Calogero, Gaetano ; Papior, Nick Rübner ; Kretz, Bernhard ; Garcia-Lekue, Aran ; Frederiksen, Thomas ; Brandbyge, Mads. / Electron transport in nanoporous graphene: Probing the Talbot effect. In: Nano letters. 2019 ; Vol. 19, No. 1. pp. 576-581.
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title = "Electron transport in nanoporous graphene: Probing the Talbot effect",
abstract = "Electrons in graphene can show diffraction and interference phenomena fully analogous to light thanks to their Dirac-like energy dispersion. However it is not clear how this optical analogy persists in nanostructured graphene, e.g. with pores. Nanoporous graphene (NPG) consisting of linked graphene nanoribbons has recently been fabricated using molecular precursors and bottom-up assembly [Moreno et al, Science 360, 199 (2018)]. We predict that electrons propagating in NPG exhibit the interference Talbot effect, analogous to photons in coupled waveguides. Our results are obtained by parameter-free atomistic calculations of real-sized NPG samples, based on seamlessly integrated density functional theory and tight-binding regions. We link the origins of this interference phenomenon to the band structure of the NPG. Most importantly, we demonstrate how the Talbot effect may be detected experimentally using dual-probe scanning tunneling microscopy. Talbot interference of electron waves in NPG or other related materials may open up new opportunities for future quantum electronics, computing or sensing.",
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author = "Gaetano Calogero and Papior, {Nick R{\"u}bner} and Bernhard Kretz and Aran Garcia-Lekue and Thomas Frederiksen and Mads Brandbyge",
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doi = "10.1021/acs.nanolett.8b04616",
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Electron transport in nanoporous graphene: Probing the Talbot effect. / Calogero, Gaetano; Papior, Nick Rübner; Kretz, Bernhard; Garcia-Lekue, Aran; Frederiksen, Thomas; Brandbyge, Mads.

In: Nano letters, Vol. 19, No. 1, 2019, p. 576-581.

Research output: Contribution to journalJournal articleResearchpeer-review

TY - JOUR

T1 - Electron transport in nanoporous graphene: Probing the Talbot effect

AU - Calogero, Gaetano

AU - Papior, Nick Rübner

AU - Kretz, Bernhard

AU - Garcia-Lekue, Aran

AU - Frederiksen, Thomas

AU - Brandbyge, Mads

PY - 2019

Y1 - 2019

N2 - Electrons in graphene can show diffraction and interference phenomena fully analogous to light thanks to their Dirac-like energy dispersion. However it is not clear how this optical analogy persists in nanostructured graphene, e.g. with pores. Nanoporous graphene (NPG) consisting of linked graphene nanoribbons has recently been fabricated using molecular precursors and bottom-up assembly [Moreno et al, Science 360, 199 (2018)]. We predict that electrons propagating in NPG exhibit the interference Talbot effect, analogous to photons in coupled waveguides. Our results are obtained by parameter-free atomistic calculations of real-sized NPG samples, based on seamlessly integrated density functional theory and tight-binding regions. We link the origins of this interference phenomenon to the band structure of the NPG. Most importantly, we demonstrate how the Talbot effect may be detected experimentally using dual-probe scanning tunneling microscopy. Talbot interference of electron waves in NPG or other related materials may open up new opportunities for future quantum electronics, computing or sensing.

AB - Electrons in graphene can show diffraction and interference phenomena fully analogous to light thanks to their Dirac-like energy dispersion. However it is not clear how this optical analogy persists in nanostructured graphene, e.g. with pores. Nanoporous graphene (NPG) consisting of linked graphene nanoribbons has recently been fabricated using molecular precursors and bottom-up assembly [Moreno et al, Science 360, 199 (2018)]. We predict that electrons propagating in NPG exhibit the interference Talbot effect, analogous to photons in coupled waveguides. Our results are obtained by parameter-free atomistic calculations of real-sized NPG samples, based on seamlessly integrated density functional theory and tight-binding regions. We link the origins of this interference phenomenon to the band structure of the NPG. Most importantly, we demonstrate how the Talbot effect may be detected experimentally using dual-probe scanning tunneling microscopy. Talbot interference of electron waves in NPG or other related materials may open up new opportunities for future quantum electronics, computing or sensing.

KW - Nanoporous graphene

KW - Talbot interference

KW - Electron transport

KW - Scanning probe microscopy

KW - Multiscale modeling

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JF - Nano Letters

SN - 1530-6984

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