Disclosing the response of the surface electronic structure in SrTiO3 (001) to strain

Eduardo Bonini Guedes, Tobias Willemoes Jensen, Muntaser Naamneh, Alla Chikina, Ramus T. Dahm, Shinhee Yun, Francesco M. Chiabrera, Nicholas C. Plumb, J. Hugo Dil, Ming Shi, Dennis Valbjørn Christensen, Walber Hugo Brito, Nini Pryds, Milan Radović

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Combining angle-resolved photoemission spectroscopy and density functional theory calculations, we addressed the surface electronic structure of bent SrTiO3 (STO) (001) wafers. Using a custom-made device, we observe that the low-dimensional states that emerge at the STO (001) surface are robust to an external tensile strain of about 0.1%. Our results show that this value of strain is too small to sensibly alter the surface conduction band of STO, but, surprisingly, it is enough to shift the energy of the in-gap states. In order to access higher strain values of around 2%, standard for STO-based heterostructures, we performed density functional theory calculations of STO slabs under different strain configurations. The simulations predict that such levels of both compressive and tensile strain significantly alter the orbital splitting of the surface conduction band. Our study indicates that the strain generated in STO can tailor the electronic properties of its bare surface and of STO-based interfaces.
Original languageEnglish
Article number013213
JournalJournal of Vacuum Science & Technology. A. Vacuum, Surfaces, and Films
Issue number1
Number of pages8
Publication statusPublished - 2022

Bibliographical note

This paper is a part of the Special Collection Honoring Dr. Scott Chambers' 70th Birthday and His Leadership in the
Science and Technology of Oxide Thin Films.


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