Compressive imaging of transient absorption dynamics on the femtosecond timescale

Ondřej Denk, Kaibo Zheng, Donatas Zigmantas, Karel Žídek*

*Corresponding author for this work

Research output: Contribution to journalJournal articleResearchpeer-review

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Abstract

Femtosecond spectroscopy is an important tool for tracking rapid photoinduced processes in a variety of materials. To spatially map the processes in a sample would substantially expand the capabilities of the method. This is, however, difficult to achieve due to the necessity to use low-noise detection and to maintain feasible data acquisition time. Here we demonstrate realization of an imaging pump-probe setup, featuring sub-100 fs temporal resolution, by a straightforward modification of a standard pump-probe technique, using a randomly structured probe beam. The structured beam, made by a diffuser, enabled us to computationally reconstruct the maps of transient absorption dynamics based on the concept of compressed sensing. We demonstrate the functionality of the setup in two proof-of-principle experiments, were we achieve spatial resolution of 20 μm. The presented concept provides a feasible route to imaging, using the pump-probe technique and ultrafast spectroscopy in general.
Original languageEnglish
JournalOptics Express
Volume27
Issue number7
Pages (from-to)10234-10246
Number of pages13
ISSN1094-4087
DOIs
Publication statusPublished - 2019

Cite this

Denk, Ondřej ; Zheng, Kaibo ; Zigmantas, Donatas ; Žídek, Karel. / Compressive imaging of transient absorption dynamics on the femtosecond timescale. In: Optics Express. 2019 ; Vol. 27, No. 7. pp. 10234-10246.
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Compressive imaging of transient absorption dynamics on the femtosecond timescale. / Denk, Ondřej; Zheng, Kaibo; Zigmantas, Donatas; Žídek, Karel.

In: Optics Express, Vol. 27, No. 7, 2019, p. 10234-10246.

Research output: Contribution to journalJournal articleResearchpeer-review

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AU - Zigmantas, Donatas

AU - Žídek, Karel

PY - 2019

Y1 - 2019

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AB - Femtosecond spectroscopy is an important tool for tracking rapid photoinduced processes in a variety of materials. To spatially map the processes in a sample would substantially expand the capabilities of the method. This is, however, difficult to achieve due to the necessity to use low-noise detection and to maintain feasible data acquisition time. Here we demonstrate realization of an imaging pump-probe setup, featuring sub-100 fs temporal resolution, by a straightforward modification of a standard pump-probe technique, using a randomly structured probe beam. The structured beam, made by a diffuser, enabled us to computationally reconstruct the maps of transient absorption dynamics based on the concept of compressed sensing. We demonstrate the functionality of the setup in two proof-of-principle experiments, were we achieve spatial resolution of 20 μm. The presented concept provides a feasible route to imaging, using the pump-probe technique and ultrafast spectroscopy in general.

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