TY - JOUR
T1 - Absolute environmental sustainability assessment of renewable dimethyl ether fuelled heavy-duty trucks
AU - Charalambous, Margarita A.
AU - Tulus, Victor
AU - Ryberg, Morten W.
AU - Pérez-Ramírez, Javier
AU - Guillén-Gosálbez, Gonzalo
N1 - Publisher Copyright:
© 2023 The Royal Society of Chemistry
PY - 2023
Y1 - 2023
N2 - In recent years, liquid fuels from renewable carbon that can replace fossil ones with minimal infrastructure changes have attracted increasing interest in decarbonising the heavy-duty long-haul sector. Here we focus on dimethyl ether (DME), a promising alternative to diesel due to its high cetane number, oxygen content, and more efficient and cleaner propulsion that results in low particulate matter and sulphur oxide emissions. Going well beyond previous studies that quantified the environmental impact of DME, often in terms of global warming, here we evaluate DME use in heavy-duty trucks in the context of seven planetary boundaries, all essential for maintaining the Earth's stability. Focusing on several scenarios differing in the feedstock origin, we find that routes based on fossil carbon, either in the form of coal, natural gas, or captured CO2 from fossil plants, would increase the greenhouse gas emissions relative to the business-as-usual. Only scenarios based on renewable carbon could reduce the impacts on climate change, while hydrogen from biomass gasification coupled with carbon capture and storage (CCS) and DME from biomass gasification with CCS could enable an environmentally sustainable operation within all the planetary boundaries. Overall, our work opens up new avenues for the environmental assessment of fuels considering the finite capacity of the Earth system to guide research and policy-making more sensibly.
AB - In recent years, liquid fuels from renewable carbon that can replace fossil ones with minimal infrastructure changes have attracted increasing interest in decarbonising the heavy-duty long-haul sector. Here we focus on dimethyl ether (DME), a promising alternative to diesel due to its high cetane number, oxygen content, and more efficient and cleaner propulsion that results in low particulate matter and sulphur oxide emissions. Going well beyond previous studies that quantified the environmental impact of DME, often in terms of global warming, here we evaluate DME use in heavy-duty trucks in the context of seven planetary boundaries, all essential for maintaining the Earth's stability. Focusing on several scenarios differing in the feedstock origin, we find that routes based on fossil carbon, either in the form of coal, natural gas, or captured CO2 from fossil plants, would increase the greenhouse gas emissions relative to the business-as-usual. Only scenarios based on renewable carbon could reduce the impacts on climate change, while hydrogen from biomass gasification coupled with carbon capture and storage (CCS) and DME from biomass gasification with CCS could enable an environmentally sustainable operation within all the planetary boundaries. Overall, our work opens up new avenues for the environmental assessment of fuels considering the finite capacity of the Earth system to guide research and policy-making more sensibly.
U2 - 10.1039/d2se01409b
DO - 10.1039/d2se01409b
M3 - Journal article
C2 - 37063612
AN - SCOPUS:85152887316
SN - 2398-4902
VL - 7
SP - 1930
EP - 1941
JO - Sustainable Energy and Fuels
JF - Sustainable Energy and Fuels
IS - 8
ER -