A Novel PDMS Dielectric Elastomer Actuator with Bis-ionic Liquid as Crosslinker

Zhaoqing Kang; Liyun Yu; Anne Ladegaard Skov

doi:10.1117/12.2610994

A Novel PDMS Dielectric Elastomer Actuator with Bis-ionic Liquid as Crosslinker

Zhaoqing Kang
, Liyun Yu
, Anne Ladegaard Skov^*

^*Corresponding author for this work

Research output: Chapter in Book/Report/Conference proceeding › Article in proceedings › Research › peer-review

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Abstract

Different from the traditional ways to prepare PDMS elastomers by addition or condensation curing reaction, a novel strategy is reported by chemical modification and curing with bis-ionic liquid (bis-IL) as a crosslinker in this study. The
IL-modified elastomer (IL-elastomer) presents a relatively low Young’s modulus of ~0.36 MPa and excellent mechanical stability with unchanged Young’s modulus and strain at break after a year. Significant improvement in relative permittivity
(εr =11 at 0.1 Hz), which is ~4 times as high as that of commercial silicone elastomers (~2.8), is proven as well. Furthermore, the dielectric elastomer actuator developed from this elastomer exhibits a maximum area strain of 9 % at 18 V/μm due to the combination of high εr and low Young’s modulus. The outstanding actuation performance of this novel elastomer suggests a promising potential for use in artificial muscles, soft robotics, and energy conversion devices.

Original language	English
Title of host publication	Electroactive Polymer Actuators and Devices (EAPAD) XXIV
Editors	Iain A. Anderson, John D. W. Madden, Herbert R. Shea
Number of pages	7
Volume	12042
Publisher	SPIE - The International Society for Optical Engineering
Publication date	2022
Article number	120420Y
DOIs	https://doi.org/10.1117/12.2610994
Publication status	Published - 2022
Event	SPIE Smart Structures + Nondestructive Evaluation 2022 - Hilton Long Beach Hotel, Long Beach, United States Duration: 6 Mar 2022 → 10 Mar 2022 https://www.spiedigitallibrary.org/conference-proceedings-of-spie/12482/1248205/Transparent-PDMS-fiber-actuator-with-ionic-liquid-based-electrodes/10.1117/12.2655769.full?SSO=1

Conference

Conference	SPIE Smart Structures + Nondestructive Evaluation 2022
Location	Hilton Long Beach Hotel
Country/Territory	United States
City	Long Beach
Period	06/03/2022 → 10/03/2022
Internet address	https://www.spiedigitallibrary.org/conference-proceedings-of-spie/12482/1248205/Transparent-PDMS-fiber-actuator-with-ionic-liquid-based-electrodes/10.1117/12.2655769.full?SSO=1

Series	Proceedings of SPIE - The International Society for Optical Engineering
ISSN	0277-786X

Keywords

Dielectric elastomer
Ionic liquid
Actuator
High permittivity
Stability

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10.1117/12.2610994

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Kang, Zhaoqing ; Yu, Liyun ; Skov, Anne Ladegaard. / A Novel PDMS Dielectric Elastomer Actuator with Bis-ionic Liquid as Crosslinker. Electroactive Polymer Actuators and Devices (EAPAD) XXIV. editor / Iain A. Anderson ; John D. W. Madden ; Herbert R. Shea. Vol. 12042 SPIE - The International Society for Optical Engineering, 2022. (Proceedings of SPIE - The International Society for Optical Engineering).

@inproceedings{232f4ba66bef44ea95ff9ed0257b9202,

title = "A Novel PDMS Dielectric Elastomer Actuator with Bis-ionic Liquid as Crosslinker",

abstract = "Different from the traditional ways to prepare PDMS elastomers by addition or condensation curing reaction, a novel strategy is reported by chemical modification and curing with bis-ionic liquid (bis-IL) as a crosslinker in this study. The IL-modified elastomer (IL-elastomer) presents a relatively low Young{\textquoteright}s modulus of \textasciitilde{}0.36 MPa and excellent mechanical stability with unchanged Young{\textquoteright}s modulus and strain at break after a year. Significant improvement in relative permittivity (εr =11 at 0.1 Hz), which is \textasciitilde{}4 times as high as that of commercial silicone elastomers (\textasciitilde{}2.8), is proven as well. Furthermore, the dielectric elastomer actuator developed from this elastomer exhibits a maximum area strain of 9 \% at 18 V/μm due to the combination of high εr and low Young{\textquoteright}s modulus. The outstanding actuation performance of this novel elastomer suggests a promising potential for use in artificial muscles, soft robotics, and energy conversion devices.",

keywords = "Dielectric elastomer, Ionic liquid, Actuator, High permittivity, Stability",

author = "Zhaoqing Kang and Liyun Yu and Skov, \{Anne Ladegaard\}",

year = "2022",

doi = "10.1117/12.2610994",

language = "English",

volume = "12042",

series = "Proceedings of SPIE - The International Society for Optical Engineering",

publisher = "SPIE - The International Society for Optical Engineering",

editor = "Anderson, \{Iain A. \} and Madden, \{John D. W. \} and Shea, \{Herbert R. \}",

booktitle = "Electroactive Polymer Actuators and Devices (EAPAD) XXIV",

note = "SPIE Smart Structures + Nondestructive Evaluation 2022 ; Conference date: 06-03-2022 Through 10-03-2022",

url = "https://www.spiedigitallibrary.org/conference-proceedings-of-spie/12482/1248205/Transparent-PDMS-fiber-actuator-with-ionic-liquid-based-electrodes/10.1117/12.2655769.full?SSO=1",

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Kang, Z, Yu, L & Skov, AL 2022, A Novel PDMS Dielectric Elastomer Actuator with Bis-ionic Liquid as Crosslinker. in IA Anderson, JDW Madden & HR Shea (eds), Electroactive Polymer Actuators and Devices (EAPAD) XXIV. vol. 12042, 120420Y, SPIE - The International Society for Optical Engineering, Proceedings of SPIE - The International Society for Optical Engineering, SPIE Smart Structures + Nondestructive Evaluation 2022, Long Beach, California, United States, 06/03/2022. https://doi.org/10.1117/12.2610994

A Novel PDMS Dielectric Elastomer Actuator with Bis-ionic Liquid as Crosslinker. / Kang, Zhaoqing; Yu, Liyun ; Skov, Anne Ladegaard.
Electroactive Polymer Actuators and Devices (EAPAD) XXIV. ed. / Iain A. Anderson; John D. W. Madden; Herbert R. Shea. Vol. 12042 SPIE - The International Society for Optical Engineering, 2022. 120420Y (Proceedings of SPIE - The International Society for Optical Engineering).

Research output: Chapter in Book/Report/Conference proceeding › Article in proceedings › Research › peer-review

TY - GEN

T1 - A Novel PDMS Dielectric Elastomer Actuator with Bis-ionic Liquid as Crosslinker

AU - Kang, Zhaoqing

AU - Yu, Liyun

AU - Skov, Anne Ladegaard

PY - 2022

Y1 - 2022

N2 - Different from the traditional ways to prepare PDMS elastomers by addition or condensation curing reaction, a novel strategy is reported by chemical modification and curing with bis-ionic liquid (bis-IL) as a crosslinker in this study. The IL-modified elastomer (IL-elastomer) presents a relatively low Young’s modulus of ~0.36 MPa and excellent mechanical stability with unchanged Young’s modulus and strain at break after a year. Significant improvement in relative permittivity (εr =11 at 0.1 Hz), which is ~4 times as high as that of commercial silicone elastomers (~2.8), is proven as well. Furthermore, the dielectric elastomer actuator developed from this elastomer exhibits a maximum area strain of 9 % at 18 V/μm due to the combination of high εr and low Young’s modulus. The outstanding actuation performance of this novel elastomer suggests a promising potential for use in artificial muscles, soft robotics, and energy conversion devices.

AB - Different from the traditional ways to prepare PDMS elastomers by addition or condensation curing reaction, a novel strategy is reported by chemical modification and curing with bis-ionic liquid (bis-IL) as a crosslinker in this study. The IL-modified elastomer (IL-elastomer) presents a relatively low Young’s modulus of ~0.36 MPa and excellent mechanical stability with unchanged Young’s modulus and strain at break after a year. Significant improvement in relative permittivity (εr =11 at 0.1 Hz), which is ~4 times as high as that of commercial silicone elastomers (~2.8), is proven as well. Furthermore, the dielectric elastomer actuator developed from this elastomer exhibits a maximum area strain of 9 % at 18 V/μm due to the combination of high εr and low Young’s modulus. The outstanding actuation performance of this novel elastomer suggests a promising potential for use in artificial muscles, soft robotics, and energy conversion devices.

KW - Dielectric elastomer

KW - Ionic liquid

KW - Actuator

KW - High permittivity

KW - Stability

U2 - 10.1117/12.2610994

DO - 10.1117/12.2610994

M3 - Article in proceedings

VL - 12042

T3 - Proceedings of SPIE - The International Society for Optical Engineering

BT - Electroactive Polymer Actuators and Devices (EAPAD) XXIV

A2 - Anderson, Iain A.

A2 - Madden, John D. W.

A2 - Shea, Herbert R.

PB - SPIE - The International Society for Optical Engineering

T2 - SPIE Smart Structures + Nondestructive Evaluation 2022

Y2 - 6 March 2022 through 10 March 2022

ER -

Kang Z, Yu L , Skov AL. A Novel PDMS Dielectric Elastomer Actuator with Bis-ionic Liquid as Crosslinker. In Anderson IA, Madden JDW, Shea HR, editors, Electroactive Polymer Actuators and Devices (EAPAD) XXIV. Vol. 12042. SPIE - The International Society for Optical Engineering. 2022. 120420Y. (Proceedings of SPIE - The International Society for Optical Engineering). doi: 10.1117/12.2610994

A Novel PDMS Dielectric Elastomer Actuator with Bis-ionic Liquid as Crosslinker

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Conference

Keywords

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