2022 roadmap on low temperature electrochemical CO2 reduction

Ifan E.L. Stephens; Karen Chan; Alexander Bagger; Shannon W. Boettcher; Julien Bonin; Etienne Boutin; Aya K. Buckley; Raffaella Buonsanti; Etosha R. Cave; Xiaoxia Chang; See Wee Chee; Alisson H.M. da Silva; Phil de Luna; Oliver Einsle; Balázs Endrődi; Maria Escudero-Escribano; Jorge V. Ferreira de Araujo; Marta C. Figueiredo; Christopher Hahn; Kentaro U. Hansen; Sophia Haussener; Sara Hunegnaw; Ziyang Huo; Yun Jeong Hwang; Csaba Janáky; Buddhinie S. Jayathilake; Feng Jiao; Zarko P. Jovanov; Parisa Karimi; Marc T.M. Koper; Kendra P. Kuhl; Woong Hee Lee; Zhiqin Liang; Xuan Liu; Sichao Ma; Ming Ma; Hyung Suk Oh; Marc Robert; Beatriz Roldan Cuenya; Jan Rossmeisl; Claudie Roy; Mary P. Ryan; Edward H. Sargent; Paula Sebastián-Pascual; Brian Seger; Ludmilla Steier; Peter Strasser; Ana Sofia Varela; Rafaël E. Vos; Xue Wang; Bingjun Xu; Hossein Yadegari; Yuxiang Zhou

doi:10.1088/2515-7655/ac7823

2022 roadmap on low temperature electrochemical CO₂ reduction

Ifan E.L. Stephens^*, Karen Chan, Alexander Bagger, Shannon W. Boettcher, Julien Bonin, Etienne Boutin, Aya K. Buckley, Raffaella Buonsanti, Etosha R. Cave, Xiaoxia Chang, See Wee Chee, Alisson H.M. da Silva, Phil de Luna, Oliver Einsle, Balázs Endrődi, Maria Escudero-Escribano, Jorge V. Ferreira de Araujo, Marta C. Figueiredo, Christopher Hahn, Kentaro U. HansenSophia Haussener, Sara Hunegnaw, Ziyang Huo, Yun Jeong Hwang, Csaba Janáky, Buddhinie S. Jayathilake, Feng Jiao, Zarko P. Jovanov, Parisa Karimi, Marc T.M. Koper, Kendra P. Kuhl, Woong Hee Lee, Zhiqin Liang, Xuan Liu, Sichao Ma, Ming Ma, Hyung Suk Oh, Marc Robert, Beatriz Roldan Cuenya, Jan Rossmeisl, Claudie Roy, Mary P. Ryan, Edward H. Sargent, Paula Sebastián-Pascual, Brian Seger, Ludmilla Steier, Peter Strasser, Ana Sofia Varela, Rafaël E. Vos, Xue Wang, Bingjun Xu, Hossein Yadegari, Yuxiang Zhou

^*Corresponding author for this work

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Abstract

Electrochemical CO₂ reduction (CO₂R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO₂R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.

Original language	English
Article number	042003
Journal	JPhys Energy
Volume	4
Issue number	4
Number of pages	85
ISSN	2515-7655
DOIs	https://doi.org/10.1088/2515-7655/ac7823
Publication status	Published - 2022

Keywords

CO2 reduction
Electrocatalysis
Electrochemistry
Solar fuels

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1088/2515-7655/ac7823

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Stephens, I. E. L., Chan, K., Bagger, A., Boettcher, S. W., Bonin, J., Boutin, E., Buckley, A. K., Buonsanti, R., Cave, E. R., Chang, X., Chee, S. W., da Silva, A. H. M., de Luna, P., Einsle, O., Endrődi, B., Escudero-Escribano, M., Ferreira de Araujo, J. V., Figueiredo, M. C., Hahn, C., ... Zhou, Y. (2022). 2022 roadmap on low temperature electrochemical CO₂ reduction. JPhys Energy, 4(4), Article 042003. https://doi.org/10.1088/2515-7655/ac7823

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author = "Stephens, {Ifan E.L.} and Karen Chan and Alexander Bagger and Boettcher, {Shannon W.} and Julien Bonin and Etienne Boutin and Buckley, {Aya K.} and Raffaella Buonsanti and Cave, {Etosha R.} and Xiaoxia Chang and Chee, {See Wee} and {da Silva}, {Alisson H.M.} and {de Luna}, Phil and Oliver Einsle and Bal{\'a}zs Endr{\H o}di and Maria Escudero-Escribano and {Ferreira de Araujo}, {Jorge V.} and Figueiredo, {Marta C.} and Christopher Hahn and Hansen, {Kentaro U.} and Sophia Haussener and Sara Hunegnaw and Ziyang Huo and Hwang, {Yun Jeong} and Csaba Jan{\'a}ky and Jayathilake, {Buddhinie S.} and Feng Jiao and Jovanov, {Zarko P.} and Parisa Karimi and Koper, {Marc T.M.} and Kuhl, {Kendra P.} and Lee, {Woong Hee} and Zhiqin Liang and Xuan Liu and Sichao Ma and Ming Ma and Oh, {Hyung Suk} and Marc Robert and Cuenya, {Beatriz Roldan} and Jan Rossmeisl and Claudie Roy and Ryan, {Mary P.} and Sargent, {Edward H.} and Paula Sebasti{\'a}n-Pascual and Brian Seger and Ludmilla Steier and Peter Strasser and Varela, {Ana Sofia} and Vos, {Rafa{\"e}l E.} and Xue Wang and Bingjun Xu and Hossein Yadegari and Yuxiang Zhou",

note = "Publisher Copyright: {\textcopyright} 2022 The Author(s). Published by IOP Publishing Ltd.",

year = "2022",

doi = "10.1088/2515-7655/ac7823",

language = "English",

volume = "4",

journal = "JPhys Energy",

issn = "2515-7655",

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Stephens, IEL, Chan, K, Bagger, A, Boettcher, SW, Bonin, J, Boutin, E, Buckley, AK, Buonsanti, R, Cave, ER, Chang, X, Chee, SW, da Silva, AHM, de Luna, P, Einsle, O, Endrődi, B, Escudero-Escribano, M, Ferreira de Araujo, JV, Figueiredo, MC, Hahn, C, Hansen, KU, Haussener, S, Hunegnaw, S, Huo, Z, Hwang, YJ, Janáky, C, Jayathilake, BS, Jiao, F, Jovanov, ZP, Karimi, P, Koper, MTM, Kuhl, KP, Lee, WH, Liang, Z, Liu, X, Ma, S, Ma, M, Oh, HS, Robert, M, Cuenya, BR, Rossmeisl, J, Roy, C, Ryan, MP, Sargent, EH, Sebastián-Pascual, P, Seger, B, Steier, L, Strasser, P, Varela, AS, Vos, RE, Wang, X, Xu, B, Yadegari, H & Zhou, Y 2022, '2022 roadmap on low temperature electrochemical CO₂ reduction', JPhys Energy, vol. 4, no. 4, 042003. https://doi.org/10.1088/2515-7655/ac7823

TY - JOUR

T1 - 2022 roadmap on low temperature electrochemical CO2 reduction

AU - Stephens, Ifan E.L.

AU - Chan, Karen

AU - Bagger, Alexander

AU - Boettcher, Shannon W.

AU - Bonin, Julien

AU - Boutin, Etienne

AU - Buckley, Aya K.

AU - Buonsanti, Raffaella

AU - Cave, Etosha R.

AU - Chang, Xiaoxia

AU - Chee, See Wee

AU - da Silva, Alisson H.M.

AU - de Luna, Phil

AU - Einsle, Oliver

AU - Endrődi, Balázs

AU - Escudero-Escribano, Maria

AU - Ferreira de Araujo, Jorge V.

AU - Figueiredo, Marta C.

AU - Hahn, Christopher

AU - Hansen, Kentaro U.

AU - Haussener, Sophia

AU - Hunegnaw, Sara

AU - Huo, Ziyang

AU - Hwang, Yun Jeong

AU - Janáky, Csaba

AU - Jayathilake, Buddhinie S.

AU - Jiao, Feng

AU - Jovanov, Zarko P.

AU - Karimi, Parisa

AU - Koper, Marc T.M.

AU - Kuhl, Kendra P.

AU - Lee, Woong Hee

AU - Liang, Zhiqin

AU - Liu, Xuan

AU - Ma, Sichao

AU - Ma, Ming

AU - Oh, Hyung Suk

AU - Robert, Marc

AU - Cuenya, Beatriz Roldan

AU - Rossmeisl, Jan

AU - Roy, Claudie

AU - Ryan, Mary P.

AU - Sargent, Edward H.

AU - Sebastián-Pascual, Paula

AU - Seger, Brian

AU - Steier, Ludmilla

AU - Strasser, Peter

AU - Varela, Ana Sofia

AU - Vos, Rafaël E.

AU - Wang, Xue

AU - Xu, Bingjun

AU - Yadegari, Hossein

AU - Zhou, Yuxiang

PY - 2022

Y1 - 2022

N2 - Electrochemical CO2 reduction (CO2R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO2R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.

AB - Electrochemical CO2 reduction (CO2R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO2R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.

KW - CO2 reduction

KW - Electrocatalysis

KW - Electrochemistry

KW - Solar fuels

U2 - 10.1088/2515-7655/ac7823

DO - 10.1088/2515-7655/ac7823

M3 - Journal article

AN - SCOPUS:85139404957

SN - 2515-7655

VL - 4

JO - JPhys Energy

JF - JPhys Energy

IS - 4

M1 - 042003

ER -