Lars David Aili

2025

Chemistry and Electrochemistry | Aluminum

Li, Q., Gao, B. & Aili, D., 2025, Encyclopedia of Electrochemical Power Sources. Garche, J. (ed.). 2 ed. Elsevier, Vol. 1. p. 585-597 13 p.

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Physicochemical properties of short-side-chain perfluorosulfonic acid membranes at elevated temperatures

Harilal, Kao, Y.-L., Pan, C., Aili, D. & Li, Q., 2025, In: Solid State Ionics. 419, 10 p., 116747.

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Reinforced Polybenzimidazole Membranes by Crosslinked Fiber Mats for High Temperature Polymer Electrolyte Membrane Fuel Cells

Chen, Y., Aili, D., Zhang, W., Azizi, K., Cleemann, L. N. & Li, Q., 2025, In: Electrochimica Acta. 529, 8 p., 146260.

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Sulfonated para-Polybenzimidazole Membranes for Use in Vanadium Redox Flow Batteries

Bui, T. T., Shin, M., Abbas, S., Ikhsan, M. M., Do, X. H., Dayan, A., Almind, M. R., Park, S., Aili, D., Hjelm, J., Hwang, J., Ha, H. Y., Azizi, K., Kwon, Y. & Henkensmeier, D., 2025, (Accepted/In press) In: Advanced Energy Materials. 10 p.

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2024

Anion exchange membranes derived from poly(ionic liquid) of poly(bis-piperidinium) and polybenzimidazole blends

Zhao, B., Wang, T., Kraglund, M. R., Yang, J., Dong, J., Tang, A., Aili, D. & Yang, J., 2024, In: Journal of Molecular Liquids. 402, 10 p., 124775.

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Bipolar Membranes Via Divergent Synthesis: On the Interplay between Ion Exchange Capacity and Water Dissociation Catalysis

Kao, Y.-L., Buchauer, F., Serhiichuk, D., Boettcher, S. W. & Aili, D., 2024, In: ACS Applied Materials and Interfaces. 16, 43, p. 58637-58647 11 p.

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Carboxylated Polystyrene-b-poly(ethylene-ran-butylene)-b-polystyrene Membranes for Alkaline Water Electrolysis

Serhiichuk, D., Tian, D., Almind, M. R., Ma, Z., Xia, Y., Kraglund, M. R., Bae, C., Jensen, J. O. & Aili, D., 2024, In: ACS Applied Energy Materials. 7, 3, p. 1080-1091 12 p.

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Divergent Synthesis of Bipolar Membranes Combining Strong Interfacial Adhesion and High-Rate Capability

Kao, Y. L., Chen, L., Boettcher, S. W. & Aili, D., 2024, In: ACS Energy Letters. 9, 6, p. 2953-2959 7 p.

Research output: Contribution to journal › Letter › peer-review

Macromolecular reinforcement of alkaline ion-solvating polymer electrolytes

Xia, Y., Abu Sara, B., Rajappan, S. C., Serhiichuk, D., Kraglund, M. R., Jensen, J. O., Deimede, V. & Aili, D., 2024, In: Polymer. 302, 9 p., 127068.

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Poly(Arylene Alkylene)s with Tetrazole Pendants for Alkaline Ion-Solvating Polymer Electrolytes

Xia, Y., Rajappan, S. C., Chen, S., Kraglund, M. R., Serhiichuk, D., Pan, D., Jensen, J. O., Jannasch, P. & Aili, D., 2024, In: ChemSusChem. 17, 23, 11 p., e202400844.

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Review and Prospects of PEM Water Electrolysis at Elevated Temperature Operation

Bonanno, M., Müller, K., Bensmann, B., Hanke‐Rauschenbach, R., Aili, D., Franken, T., Chromik, A., Peach, R., Freiberg, A. T. S. & Thiele, S., 2024, In: Advanced Materials Technologies. 9, 2, 25 p., 2300281.

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Separators and Membranes for Advanced Alkaline Water Electrolysis

Henkensmeier, D., Cho, W.-C., Jannasch, P., Stojadinovic, J., Li, Q., Aili, D. & Jensen, J. O., 2024, In: Chemical Reviews. 124, 10, p. 6393-6443 51 p.

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Tetrazole functionalization: a new strategy toward stable alkaline ion-solvating polymer electrolytes

Serhiichuk, D., Rajappan, S. C., Krishnan, Y., Xia, Y., Kraglund, M. R., Hansen, H. A., Jensen, J. O. & Aili, D., 2024, In: Journal of Materials Chemistry A. 12, 47, p. 32697-32702 6 p.

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2023

Electrode Separators for the Next-Generation Alkaline Water Electrolyzers

Aili, D., Kraglund, M. R., Rajappan, S. C., Serhiichuk, D., Xia, Y., Deimede, V., Kallitsis, J., Bae, C., Jannasch, P., Henkensmeier, D. & Jensen, J. O., 2023, In: ACS Energy Letters. 8, 4, p. 1900-1910 11 p.

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Insight into the Alkaline Stability of Arylene-Linked Bis-Benzimidazoles and Polybenzimidazoles

Serhiichuk, D., Patniboon, T., Xia, Y., Kraglund, M. R., Jensen, J. O., Hansen, H. A. & Aili, D., 2023, In: ACS Applied Polymer Materials. 5, 1, p. 803-814 12 p.

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Performance degradation and mitigation of high temperature polybenzimidazole-based polymer electrolyte membrane fuel cells

Seselj, N., Aili, D., Celenk, S., Cleemann, L. N., Hjuler, H. A., Jensen, J. O., Azizi, K. & Li, Q., 2023, In: Chemical Society Reviews. 52, p. 4046-4070 25 p.

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Poly(vinyl alcohol-co-vinyl acetal) gel electrolytes for alkaline water electrolysis

Xia, Y., Rajappan, S., Serhiichuk, D., Kraglund, M. R., Jensen, J. O. & Aili, D., 2023, In: Journal of Membrane Science. 680, 10 p., 121719.

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Polyisatin derived ion-solvating blend membranes for alkaline water electrolysis

Makrygianni, M., Aivali, S., Xia, Y., Kraglund, M. R., Aili, D. & Deimede, V., 2023, In: Journal of Membrane Science. 669, 12 p., 121331.

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Quaternary Ammonium-Free Membranes for Water Electrolysis with 1 m KOH

Dayan, A., Trisno, M. L. A., Yang, C., Kraglund, M. R., Almind, M. R., Hjelm, J., Jensen, J. O., Aili, D., Park, H. S. & Henkensmeier, D., 2023, In: Advanced Energy Materials. 13, 46, 10 p., 2302966.

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Tuning Polybenzimidazole-Derived Crosslinked Interpenetrating Network Membranes for Vanadium Redox Flow Batteries

Pasadakis-Kavounis, A., Arslan, F., Almind, M. R., Aili, D. & Hjelm, J., 2023, In: Batteries and Supercaps. 6, 9, 9 p., e202300176.

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2022

An Imidazolium Type Ionic Liquid Functionalized Ether-Free Poly(terphenyl piperidinium) Membrane for High Temperature Polymer Electrolyte Membrane Fuel Cell Applications

Jin, Y., Che, X., Xu, Y., Dong, J., Pan, C., Aili, D., Li, Q. & Yang, J., 2022, In: Journal of the Electrochemical Society. 169, 2, 8 p., 024504.

Research output: Contribution to journal › Journal article › Research › peer-review

Anion conductivity of cation exchange membranes in aqueous supporting electrolytes

Tang, H., Aili, D., Tufa, R. A., Kraglund, M. R., Wu, Q., Pan, C., Cleemann, L. N. & Li, Q., 2022, In: Solid State Ionics. 383, 8 p., 115984.

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Anion exchange membranes based on long side-chain quaternary ammonium-functionalized poly(arylene piperidinium)s for vanadium redox flow batteries

Che, X., Tang, W., Dong, J., Aili, D. & Yang, J., 2022, In: Science China Materials. 65, 3, p. 683–694 12 p.

Research output: Contribution to journal › Journal article › Research › peer-review

Bipolar polymer electrolyte membranes for electrochemical CO₂ conversion

Kao, Y.-L., Tufa, R. & Aili, D., 2022, 3rd International Conference on Electrolysis: Book of Abstracts. 2 p. 43

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Electroreduction of CO₂ to ethanol by electrochemically deposited Cu-lignin complexes on Ni foam electrodes

Chanda, D., Tufa, R. A., Aili, D. & Basu, S., 2022, In: Nanotechnology. 33, 11 p., 055403.

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Feasibility of using thin polybenzimidazole electrolytes in high-temperature proton exchange membrane fuel cells

Chen, Y., Azizi, K., Zhang, W., Aili, D., Primdahl, S., Cleemann, L. N., Hjuler, H. A. & Li, Q., 2022, In: International Journal of Hydrogen Energy. 47, 66, p. 28615-28625 11 p.

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Low Pt loading for high-performance fuel cell electrodes enabled by hydrogen-bonding microporous polymer binders

Tang, H., Geng, K., Aili, D., Ju, Q., Pan, J., Chao, G., Yin, X., Guo, X., Li, Q. & Li, N., 2022, In: Nature Communications. 13, 1, 13 p., 7577.

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Perspectives of ion-solvating membranes for alkaline electrolysis

Jensen, J. O., Kraglund, M. R., Gellrich, F., Serhiichuk, D., Xia, Y., Chatzichristodoulou, C., Li, Q. & Aili, D., 2022, 3rd International Conference on Electrolysis: Book of Abstracts. 2 p. 108

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Reinforced gel-state polybenzimidazole hydrogen separators for alkaline water electrolysis

Trisno, M. L. A., Dayan, A., Lee, S. J., Egert, F., Gerle, M., Kraglund, M. R., Jensen, J. O., Aili, D., Roznowska, A., Michalak, A., Park, H. S., Razmjooei, F., Ansar, S.-A. & Henkensmeier, D., 2022, In: Energy and Environmental Science. 15, 10, p. 4362-4375 14 p.

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2021

Bipolar Membrane and Interface Materials for Electrochemical Energy Systems

Tufa, R. A., Blommaert, M. A., Chanda, D., Li, Q., Vermaas, D. A. & Aili, D., 2021, In: ACS Applied Energy Materials. 4, 8, p. 7419-7439 21 p.

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Diamine crosslinked anion exchange membranes based on poly(vinyl benzyl methylpyrrolidinium) for alkaline water electrolysis

Li, H., Yu, N., Gellrich, F., Reumert, A. K., Kraglund, M. R., Dong, J., Aili, D. & Yang, J., 2021, In: Journal of Membrane Science. 633, 11 p., 119418.

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Evaluation of Diaphragms and Membranes as Separators for Alkaline Water Electrolysis

Brauns, J., Schonebeck, J., Kraglund, M. R., Aili, D., Hnat, J., Zitka, J., Mues, W., Jensen, J. O., Bouzek, K. & Turek, T., 2021, In: Journal of the Electrochemical Society. 168, 1, 13 p., 014510.

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Facile synthesis and properties of poly(ether ketone cardo)s bearing heterocycle groups for high temperature polymer electrolyte membrane fuel cells

Liu, R., Wang, J., Che, X., Wang, T., Aili, D., Li, Q. & Yang, J., 2021, In: Journal of Membrane Science. 636, 9 p., 119584.

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Insights and Challenges for Applying Bipolar Membranes in Advanced Electrochemical Energy Systems

Blommaert, M. A., Aili, D., Tufa, R. A., Li, Q., Smith, W. A. & Vermaas, D. A., 2021, In: ACS Energy Letters. 6, p. 2539-2548

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On the stability of imidazolium and benzimidazolium salts in phosphoric acid based fuel cell electrolytes

Tang, H., Aili, D., Geng, K., Gao, J., Li, Q. & Li, N., 2021, In: Journal of Power Sources. 515, 9 p., 230642.

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Studies on Anion Exchange Membrane and Interface Properties by Electrochemical Impedance Spectroscopy: The Role of pH

Zhang, W., Cheng, W., Tufa, R. A., Liu, C., Aili, D., Chanda, D., Chang, J., Wang, S., Zhang, Y. & Ma, J., 2021, In: Membranes. 11, 10, 17 p., 771.

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2020

Advancement toward Polymer Electrolyte Membrane Fuel Cells at Elevated Temperatures

Zhang, J., Aili, D., Lu, S., Li, Q. & Jiang, S. P., 2020, In: Research - a science partner journal. 2020, 15 p., 9089405.

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Cationic ether-free poly(bis-alkylimidazolium) ionene blend polybenzimidazole as anion exchange membranes

Dong, J., Yu, N., Che, X., Liu, R., Aili, D. & Yang, J., 2020, In: Polymer Chemistry. 11, 37, p. 6037-6046

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From polybenzimidazoles to polybenzimidazoliums and polybenzimidazolides

Aili, D., Yang, J., Jankova, K. J., Henkensmeier, D. & Li, Q., 2020, In: Journal of Materials Chemistry A. 8, 26, p. 12854-12886

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Membranes for zinc-air batteries: Recent progress, challenges and perspectives

Tsehaye, M. T., Alloin, F., Iojoiu, C., Tufa, R. A., Aili, D., Fischer, P. & Velizarov, S., 2020, In: Journal of Power Sources. 475, 23 p., 228689.

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Phosphoric Acid Dynamics in High Temperature Polymer Electrolyte Membranes

Aili, D., Becker, H., Reimer, U., Andreasen, J. W., Cleemann, L. N., Jensen, J. O., Pan, C., Wang, X., Lehnert, W. & Li, Q., 2020, In: Journal of the Electrochemical Society. 167, 13, 8 p., 134507.

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Polybenzimidazole-Based High-Temperature Polymer Electrolyte Membrane Fuel Cells: New Insights and Recent Progress

Aili, D., Henkensmeier, D., Martin Fernandez, S., Singh, B., Hu, Y., Jensen, J. O., Cleemann, L. N. & Li, Q., 2020, In: Electrochemical Energy Reviews. 3, p. 793–845

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Polysulfone-polyvinylpyrrolidone blend membranes as electrolytes in alkaline water electrolysis

Aili, D., Kraglund, M. R., Tavacoli, J., Chatzichristodoulou, C. & Jensen, J. O., 2020, In: Journal of Membrane Science. 598, 10 p., 117674.

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Protic ionic liquids immobilized in phosphoric acid-doped polybenzimidazole matrix enable polymer electrolyte fuel cell operation at 200 °C

Skorikova, G., Rauber, D., Aili, D., Martin, S., Li, Q., Henkensmeier, D. & Hempelmann, R., 2020, In: Journal of Membrane Science. 608, 11 p., 118188.

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Three-layered electrolyte membranes with acid reservoir for prolonged lifetime of high-temperature polymer electrolyte membrane fuel cells

Kannan, A., Aili, D., Cleemann, L. N., Li, Q. & Jensen, J. O., 2020, In: International Journal of Hydrogen Energy. 45, 1, p. 1008-1017 10 p.

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Towards highly efficient electrochemical CO₂ reduction: Cell designs, membranes and electrocatalysts

Tufa, R. A., Chanda, D., Ma, M., Aili, D., Demissie, T. B., Vaes, J., Li, Q., Liu, S. & Pant, D., 2020, In: Applied Energy. 277, 115557.

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2019

Anion exchange membranes of bis-imidazolium cation crosslinked poly(2,6-dimethyl-1,4- phenylene oxide) with enhanced alkaline stability

Dong, J., Li, H., Ren, X., Che, X., Yang, J. & Aili, D., 2019, In: International Journal of Hydrogen Energy. 44, 39, p. 22137-22145

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Design of Monovalent Ion Selective Membranes for Reducing the Impacts of Multivalent Ions in Reverse Electrodialysis

Besha, A. T., Tsehaye, M. T., Aili, D., Zhang, W. & Tufa, R. A., 2019, In: Membranes. 10, 1, 28 p., 7.

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Durability and degradation of vapor-fed direct dimethyl ether high temperature polymer electrolyte membrane fuel cells

Vassiliev, A., Reumert, A. K., Jensen, J. O. & Aili, D., 2019, In: Journal of Power Sources. 432, p. 30-37

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Ion-solvating membranes as a new approach towards high rate alkaline electrolyzers

Kraglund, M. R., Carmo, M., Schiller, G., Ansar, S. A., Aili, D., Christensen, E. & Jensen, J. O., 2019, In: Energy and Environmental Science. 12, 11, p. 3313-3318 6 p.

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Lars David Aili

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