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Bibtex

@article{cad625faecc64419a9cedfd184930934,
title = "Phase-only shaped laser pulses in optimal control theory: Application to indirect photofragmentation dynamics in the weak-field limit",
keywords = "PHYSICS,, QUANTUM OPTIMAL-CONTROL, PREDISSOCIATION DYNAMICS, MOLECULAR-DYNAMICS, CHEMICAL-REACTIONS, FEMTOSECOND, PHOTODISSOCIATION, HALIDES",
publisher = "American Institute of Physics",
author = "Chuan-Cun Shu and Henriksen, {Niels E.}",
note = "Copyright (2012) American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics.",
year = "2012",
doi = "10.1063/1.3678013",
volume = "136",
number = "4",
pages = "044303",
journal = "Journal of Chemical Physics",
issn = "0021-9606",

}

RIS

TY - JOUR

T1 - Phase-only shaped laser pulses in optimal control theory: Application to indirect photofragmentation dynamics in the weak-field limit

A1 - Shu,Chuan-Cun

A1 - Henriksen,Niels E.

AU - Shu,Chuan-Cun

AU - Henriksen,Niels E.

PB - American Institute of Physics

PY - 2012

Y1 - 2012

N2 - We implement phase-only shaped laser pulses within quantum optimal control theory for laser-molecule interaction. This approach is applied to the indirect photofragmentation dynamics of NaI in the weak-field limit. It is shown that optimized phase-modulated pulses with a fixed frequency distribution can substantially modify transient dissociation probabilities as well as the momentum distribution associated with the relative motion of Na and I. © 2012 American Institute of Physics.

AB - We implement phase-only shaped laser pulses within quantum optimal control theory for laser-molecule interaction. This approach is applied to the indirect photofragmentation dynamics of NaI in the weak-field limit. It is shown that optimized phase-modulated pulses with a fixed frequency distribution can substantially modify transient dissociation probabilities as well as the momentum distribution associated with the relative motion of Na and I. © 2012 American Institute of Physics.

KW - PHYSICS,

KW - QUANTUM OPTIMAL-CONTROL

KW - PREDISSOCIATION DYNAMICS

KW - MOLECULAR-DYNAMICS

KW - CHEMICAL-REACTIONS

KW - FEMTOSECOND

KW - PHOTODISSOCIATION

KW - HALIDES

UR - http://jcp.aip.org.globalproxy.cvt.dk/resource/1/jcpsa6/v136/i4/p044303_s1

U2 - 10.1063/1.3678013

DO - 10.1063/1.3678013

JO - Journal of Chemical Physics

JF - Journal of Chemical Physics

SN - 0021-9606

IS - 4

VL - 136

SP - 044303

ER -