Particle concentration and flux dynamics in the atmospheric boundary layer as the indicator of formation mechanism

Publication: Research - peer-reviewJournal article – Annual report year: 2010

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We carried out column model simulations to study particle fluxes and deposition and to evaluate different particle formation mechanisms at a boreal forest site in Finland. We show that kinetic nucleation of sulphuric acid cannot be responsible for new particle formation alone as the vertical profile of particle number distribution does not correspond to observations. Instead organic induced nucleation leads to good agreement confirming the relevance of the aerosol formation mechanism including organic compounds emitted by biosphere. Simulation of aerosol concentration inside the atmospheric boundary layer during nucleation days shows highly dynamical picture, where particle formation is coupled with chemistry and turbulent transport. We have demonstrated suitability of our turbulent mixing scheme in reproducing most important characteristics of particle dynamics inside the atmospheric boundary layer. Deposition and particle flux simulations show that deposition affects noticeably only the smallest particles at the lowest part of the atmospheric boundary layer.
Original languageEnglish
JournalAtmospheric Chemistry and Physics Discussions
Publication date2010
Volume10
Journal number8
Pages20005-20033
ISSN1680-7367
DOIs
StatePublished
CitationsWeb of Science® Times Cited: No match on DOI

Keywords

  • Wind power meteorology, Wind Energy

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