Coherent Manipulation of a Molecular Ln-Based Nuclear Qudit Coupled to an Electron Qubit

Publication: Research - peer-reviewJournal article – Annual report year: 2018

DOI

  • Author: Hussain, Riaz

    University of Parma

  • Author: Allodi, Giuseppe

    University of Parma

  • Author: Chiesa, Alessandro

    University of Parma

  • Author: Garlatti, Elena

    University of Parma

  • Author: Mitcov, Dmitri

    University of Copenhagen

  • Author: Konstantatos, Andreas

    University of Copenhagen

  • Author: Pedersen, Kasper S.

    Organic Chemistry, Department of Chemistry, Technical University of Denmark, Kemitorvet, 2800, Kgs. Lyngby, Denmark

  • Author: De Renzi, Roberto

    University of Parma

  • Author: Piligkos, Stergios

    University of Copenhagen

  • Author: Carretta, Stefano

    University of Parma

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We demonstrate that the [Yb(trensal)] molecule is a prototypical coupled electronic qubit-nuclear qudit system. The combination of noise-resilient nuclear degrees of freedom and large reduction of nutation time induced by electron-nuclear mixing enables coherent manipulation of this qudit by radio frequency pulses. Moreover, the multilevel structure of the qudit is exploited to encode and operate a qubit with embedded basic quantum error correction.

Original languageEnglish
JournalJournal of the American Chemical Society
Volume140
Issue number31
Pages (from-to)9814-9818
ISSN0002-7863
DOIs
StatePublished - 8 Aug 2018
CitationsWeb of Science® Times Cited: 0
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